Exciton–Exciton Interaction and Optical Gain in Colloidal CdSe/CdS Dot/Rod Nanocrystals

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Abstract

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Exciton–exciton interaction in dot/rod CdSe/CdS nanocrystals has proved to be very sensitive to the shape of nanocrystals, due to the unique band alignment between CdSe and CdS. Repulsive exciton–exciton interaction is demonstrated, which makes CdSe/CdS dot/rods promising gain media for solution-processable lasers, with projected pump threshold densities below 1 kW cm−2 for continuous wave lasing.

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