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Energy-Efficient Dehumidification over Hierachically Porous Metal–Organic Frameworks as Advanced Water Adsorbents

Authors

  • You-Kyong Seo,

    1. Catalysis Center for Molecular Engineering (CCME), Korea Research Institute of Chemical Technology (KRICT), Jang-dong 100, Yuseong, Daejeon 305-600, Korea
    2. Department of Chemistry, Center for Bioactive Molecular Hybrid, Yonsei University, Seodaemoonku, Seoul 120-749, Korea
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  • Ji Woong Yoon,

    1. Catalysis Center for Molecular Engineering (CCME), Korea Research Institute of Chemical Technology (KRICT), Jang-dong 100, Yuseong, Daejeon 305-600, Korea
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  • Ji Sun Lee,

    1. Catalysis Center for Molecular Engineering (CCME), Korea Research Institute of Chemical Technology (KRICT), Jang-dong 100, Yuseong, Daejeon 305-600, Korea
    2. Department of Chemistry, Center for Bioactive Molecular Hybrid, Yonsei University, Seodaemoonku, Seoul 120-749, Korea
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  • Young Kyu Hwang,

    1. Catalysis Center for Molecular Engineering (CCME), Korea Research Institute of Chemical Technology (KRICT), Jang-dong 100, Yuseong, Daejeon 305-600, Korea
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  • Chul-Ho Jun,

    1. Department of Chemistry, Center for Bioactive Molecular Hybrid, Yonsei University, Seodaemoonku, Seoul 120-749, Korea
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  • Jong-San Chang,

    Corresponding author
    1. Catalysis Center for Molecular Engineering (CCME), Korea Research Institute of Chemical Technology (KRICT), Jang-dong 100, Yuseong, Daejeon 305-600, Korea
    • Catalysis Center for Molecular Engineering (CCME), Korea Research Institute of Chemical Technology (KRICT), Jang-dong 100, Yuseong, Daejeon 305-600, Korea.
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  • Stefan Wuttke,

    1. Laboratoire Catalyse et Spectrochimie, UMR 6506, CNRS/ENSICAEN et Université de Caen Basse-Normandie, UNICITE, 14, rue Alfred Kastler, 14052 Caen Cedex 4, France
    2. Institut Lavoisier (UMR CNRS 8180), Université de Versailles Saint-Quentin-en-Yvelines, 45 avenue des Etats-Unis, 78035 Versailles Cedex, France
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  • Philippe Bazin,

    1. Laboratoire Catalyse et Spectrochimie, UMR 6506, CNRS/ENSICAEN et Université de Caen Basse-Normandie, UNICITE, 14, rue Alfred Kastler, 14052 Caen Cedex 4, France
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  • Alexandre Vimont,

    1. Laboratoire Catalyse et Spectrochimie, UMR 6506, CNRS/ENSICAEN et Université de Caen Basse-Normandie, UNICITE, 14, rue Alfred Kastler, 14052 Caen Cedex 4, France
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  • Marco Daturi,

    1. Laboratoire Catalyse et Spectrochimie, UMR 6506, CNRS/ENSICAEN et Université de Caen Basse-Normandie, UNICITE, 14, rue Alfred Kastler, 14052 Caen Cedex 4, France
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  • Sandrine Bourrelly,

    1. Laboratoire Chimie Provence, UMR 6264 Universite's Aix-Marseille I, II & III-CNRS, Centre de St Jérôme, 13397 Marseille Cedex 20, France
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  • Philip L. Llewellyn,

    1. Laboratoire Chimie Provence, UMR 6264 Universite's Aix-Marseille I, II & III-CNRS, Centre de St Jérôme, 13397 Marseille Cedex 20, France
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  • Patricia Horcajada,

    1. Institut Lavoisier (UMR CNRS 8180), Université de Versailles Saint-Quentin-en-Yvelines, 45 avenue des Etats-Unis, 78035 Versailles Cedex, France
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  • Christian Serre,

    1. Institut Lavoisier (UMR CNRS 8180), Université de Versailles Saint-Quentin-en-Yvelines, 45 avenue des Etats-Unis, 78035 Versailles Cedex, France
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  • Gérard Férey

    1. Institut Lavoisier (UMR CNRS 8180), Université de Versailles Saint-Quentin-en-Yvelines, 45 avenue des Etats-Unis, 78035 Versailles Cedex, France
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Abstract

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Hierarchically porous metal–organic frameworks with mesoporous cages are demonstrated to behave as promising water adsorbents in energy-efficient dehumidification. Their low temperature desorption properties for water with huge sorption uptakes are essential for various water sorption applications including desiccant dehumidification and fresh water production.

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