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Non-Blinking Single-Photon Generation with Anisotropic Colloidal Nanocrystals: Towards Room-Temperature, Efficient, Colloidal Quantum Sources

Authors

  • Ferruccio Pisanello,

    Corresponding author
    1. Istituto Italiano di Tecnologia (IIT), Center for Bio-Molecular Nanotechnologies, Via Barsanti sn, 73010 Arnesano (Lecce), Italy
    2. Laboratoire Kastler Brossel, Université Pierre et Marie Curie, CNRS UMR 8552, Ecole Normale Supérieure, 4 place Jussieu, 75252 Paris Cedex 05, France
    3. Center for Neuroscience and Cognitive Systems @UNITN, Istituto Italiano di Tecnologia, corso Bettini 31, 38068 Rovereto (TN), Italy
    • Istituto Italiano di Tecnologia (IIT), Center for Bio-Molecular Nanotechnologies, Via Barsanti sn, 73010 Arnesano (Lecce), Italy.
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  • Godefroy Leménager,

    1. Laboratoire Kastler Brossel, Université Pierre et Marie Curie, CNRS UMR 8552, Ecole Normale Supérieure, 4 place Jussieu, 75252 Paris Cedex 05, France
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  • Luigi Martiradonna,

    1. Istituto Italiano di Tecnologia (IIT), Center for Bio-Molecular Nanotechnologies, Via Barsanti sn, 73010 Arnesano (Lecce), Italy
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  • Luigi Carbone,

    1. National Nanotechnology Laboratory (NNL)- CNR Istituto Nanoscienze, c/o Distretto Tecnologico, via per Arnesano km 5, 73100 Lecce, Italy
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  • Stefano Vezzoli,

    1. Laboratoire Kastler Brossel, Université Pierre et Marie Curie, CNRS UMR 8552, Ecole Normale Supérieure, 4 place Jussieu, 75252 Paris Cedex 05, France
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  • Pascal Desfonds,

    1. Laboratoire Kastler Brossel, Université Pierre et Marie Curie, CNRS UMR 8552, Ecole Normale Supérieure, 4 place Jussieu, 75252 Paris Cedex 05, France
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  • Pantaleo Davide Cozzoli,

    1. National Nanotechnology Laboratory (NNL)- CNR Istituto Nanoscienze, c/o Distretto Tecnologico, via per Arnesano km 5, 73100 Lecce, Italy
    2. Dipartimento di Matematica e Fisica “E. De Giorgi” - Università del Salento, via per Arnesano, 73100 Lecce, Italy
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  • Jean-Pierre Hermier,

    1. Groupe d'étude de la Matière Condensée, CNRS UMR8635, Université de Versailles, Saint-Quentin-en-Yvelines, 45 avenue des Etats-Unis, 78035 Versailles Cedex, France
    2. Institut Universitaire de France, 103, Boulevard Saint-Michel, F-75005, Paris, France
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  • Elisabeth Giacobino,

    1. Laboratoire Kastler Brossel, Université Pierre et Marie Curie, CNRS UMR 8552, Ecole Normale Supérieure, 4 place Jussieu, 75252 Paris Cedex 05, France
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  • Roberto Cingolani,

    1. Istituto Italiano di Tecnologia (IIT), Via Morego 30, 16163 Genova, Italy
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  • Massimo De Vittorio,

    1. Istituto Italiano di Tecnologia (IIT), Center for Bio-Molecular Nanotechnologies, Via Barsanti sn, 73010 Arnesano (Lecce), Italy
    2. National Nanotechnology Laboratory (NNL)- CNR Istituto Nanoscienze, c/o Distretto Tecnologico, via per Arnesano km 5, 73100 Lecce, Italy
    3. Dipartimento di Ingegneria dell'Innovazione - Università del, Salento, via per Monteroni, 73100 Lecce, Italy, Istituto Italiano di Tecnologia (IIT), Center for Bio-Molecular Nanotechnologies, Via Barsanti sn, 73010 Arnesano (Lecce), Italy
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  • Alberto Bramati

    1. Laboratoire Kastler Brossel, Université Pierre et Marie Curie, CNRS UMR 8552, Ecole Normale Supérieure, 4 place Jussieu, 75252 Paris Cedex 05, France
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Abstract

Blinking and single-photon emission can be tailored in CdSe/CdS core/shell colloidal dot-in-rods. By increasing the shell thickness it is possible to obtain almost non-blinking nanocrystals, while the shell length can be used to control single-photon emission probability.

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