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Electrochemical Route to Fabricate Film-Like Conjugated Microporous Polymers and Application for Organic Electronics

Authors

  • Cheng Gu,

    1. State Key Laboratory of Supramolecular, Structure and Materials, Jilin University, Qianjin Avenue, Changchun, 130012, P. R. China
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  • Youchun Chen,

    1. State Key Laboratory of Supramolecular, Structure and Materials, Jilin University, Qianjin Avenue, Changchun, 130012, P. R. China
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  • Zhongbo Zhang,

    1. State Key Laboratory of Supramolecular, Structure and Materials, Jilin University, Qianjin Avenue, Changchun, 130012, P. R. China
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  • Shanfeng Xue,

    1. State Key Laboratory of Supramolecular, Structure and Materials, Jilin University, Qianjin Avenue, Changchun, 130012, P. R. China
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  • Shuheng Sun,

    1. State Key Laboratory of Supramolecular, Structure and Materials, Jilin University, Qianjin Avenue, Changchun, 130012, P. R. China
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  • Kai Zhang,

    1. State Key Laboratory of Luminescent Materials and Devices, Institute of Polymer Optoelectronic Materials and Devices, South China University of Technology, Guangzhou 510640, P. R. China
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  • Chengmei Zhong,

    1. State Key Laboratory of Luminescent Materials and Devices, Institute of Polymer Optoelectronic Materials and Devices, South China University of Technology, Guangzhou 510640, P. R. China
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  • Huanhuan Zhang,

    1. State Key Laboratory of Supramolecular, Structure and Materials, Jilin University, Qianjin Avenue, Changchun, 130012, P. R. China
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  • Yuyu Pan,

    1. State Key Laboratory of Supramolecular, Structure and Materials, Jilin University, Qianjin Avenue, Changchun, 130012, P. R. China
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  • Ying Lv,

    1. State Key Laboratory of Supramolecular, Structure and Materials, Jilin University, Qianjin Avenue, Changchun, 130012, P. R. China
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  • Yanqin Yang,

    1. Key Laboratory of Polymer Ecomaterials, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P. R. China
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  • Fenghong Li,

    Corresponding author
    1. State Key Laboratory of Supramolecular, Structure and Materials, Jilin University, Qianjin Avenue, Changchun, 130012, P. R. China
    • State Key Laboratory of Supramolecular, Structure and Materials, Jilin University, Qianjin Avenue, Changchun, 130012, P. R. China
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  • Suobo Zhang,

    1. Key Laboratory of Polymer Ecomaterials, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, P. R. China
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  • Fei Huang,

    Corresponding author
    1. State Key Laboratory of Luminescent Materials and Devices, Institute of Polymer Optoelectronic Materials and Devices, South China University of Technology, Guangzhou 510640, P. R. China
    • State Key Laboratory of Luminescent Materials and Devices, Institute of Polymer Optoelectronic Materials and Devices, South China University of Technology, Guangzhou 510640, P. R. China.
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  • Yuguang Ma

    Corresponding author
    1. State Key Laboratory of Supramolecular, Structure and Materials, Jilin University, Qianjin Avenue, Changchun, 130012, P. R. China
    2. State Key Laboratory of Luminescent Materials and Devices, Institute of Polymer Optoelectronic Materials and Devices, South China University of Technology, Guangzhou 510640, P. R. China
    • State Key Laboratory of Supramolecular, Structure and Materials, Jilin University, Qianjin Avenue, Changchun, 130012, P. R. China
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Abstract

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Film-like conjugated microporous polymers (CMPs) are fabricated by the novel strategy of carbazole-based electropolymerization. The CMP film storing a mass of counterions acting as an anode interlayer provides a significant power-conversion efficiency of 7.56% in polymer solar cells and 20.7 cd A−1 in polymer light-emitting diodes, demonstrating its universality and potential as an electrode interlayer in organic electronics.

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