Recyclable nanocatalysts of core–shell bimetallic nanocrystals are developed through polydopamine coating-directed one-step seeded growth, interfacial assembly, and substrate-immobilization of Au@Ag core–shell nanocrystals. This strategy provides new opportunities to design and optimize heterogeneous nanocatalysts with tailored size, morphology, chemical configuration, and supporting substrates for metal-catalyzed reactions.
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