Nitrogen-Doped Holey Graphitic Carbon from 2D Covalent Organic Polymers for Oxygen Reduction

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Abstract

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Using covalent organic polymer pre­cursors, we have developed a new strategy for location control of N-dopant heteroatoms in the graphitic porous carbon, which otherwise is impossible to achieve with conventional N-doping techniques. The electrocatalytic activities of the N-doped holey graphene analogues are well correlated to the N-locations, showing possibility for tailoring the structure and property of N-doped carbon nanomaterials.

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