Advanced Synthesis & Catalysis

Cover image for Vol. 356 Issue 8

May 26, 2014

Volume 356, Issue 8

Pages 1649–1882

  1. Cover Pictures

    1. Top of page
    2. Cover Pictures
    3. Contents
    4. Corrigendum
    5. Review
    6. Communications
    7. Full Papers
    8. Updates
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      Copper-Catalyzed Decarboxylative C[TRIPLE BOND]N Triple Bond Formation: Direct Synthesis of Benzonitriles from Phenylacetic Acids Under O2 Atmosphere (page 1649)

      Qiang Feng and Qiuling Song

      Version of Record online: 18 MAR 2014 | DOI: 10.1002/adsc.201400205

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      The front cover picture, provided by Qiang Feng and Qiuling Song, illustrates a coppercatalyzed reaction of phenylacetic acids and urea to afford benzonitriles under an oxygen atmosphere. This reaction proceeds smoothly by a sequence of decarboxylation, dioxygen activation, C[BOND]H bond functionalization, and nitrile formation with urea as the nitrogen source. Molecular oxygen was found to play a crucial role in this transformation. This reaction represents a novel protocol for the formation of benzonitriles in an environmental friendly way and with good functional group tolerability, as reported in the communication on pages 1697–1702 (Q. Feng, Q. Song, Adv. Synth. Catal. 2014, 356, 1697–1702; DOI: 10.1002/adsc.201301001).

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      Chiral Phosphoric Acid-Catalyzed Enantioselective Three- Component Aza-Diels–Alder Reactions of Aminopyrroles and Aminopyrazoles (page 1888)

      Julien Brioche, Thibaut Courant, Lilian Alcaraz, Michael Stocks, Mark Furber, Jieping Zhu and Géraldine Masson

      Version of Record online: 13 MAY 2014 | DOI: 10.1002/adsc.201400456

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      The back cover picture, provided by Géraldine Masson, illustrates the straightforward three-component process catalyzed by chiral phosphoric acid. The authors reveal the first use of aminopyrroles and aminopyrazoles as partners in the asymmetric three-component Povarov reaction providing an access to novel chiral heterocyclic structures in excellent diastereoselectivities as well as good yields and enantioselectivities, as reported in the communication on pages 1719–1724 (J. Brioche, T. Courant, L. Alcaraz, M. Stocks, M. Furber, J. Zhu, G. Masson, Adv. Synth. Catal. 2014, 356, 1719–1724; DOI: 10.1002/adsc.201400093).

  2. Contents

    1. Top of page
    2. Cover Pictures
    3. Contents
    4. Corrigendum
    5. Review
    6. Communications
    7. Full Papers
    8. Updates
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  3. Corrigendum

    1. Top of page
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    3. Contents
    4. Corrigendum
    5. Review
    6. Communications
    7. Full Papers
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      Corrigendum: Carboxylate-Directed C[BOND]H Functionalization (page 1659)

      Guangfa Shi and Yanghui Zhang

      Version of Record online: 21 MAY 2014 | DOI: 10.1002/adsc.201400464

      This article corrects:

      Carboxylate-Directed C[BOND]H Functionalization

      Vol. 356, Issue 7, 1419–1442, Version of Record online: 30 APR 2014

  4. Review

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    3. Contents
    4. Corrigendum
    5. Review
    6. Communications
    7. Full Papers
    8. Updates
  5. Communications

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    4. Corrigendum
    5. Review
    6. Communications
    7. Full Papers
    8. Updates
    1. Modular Synthesis of Ar-BINMOL-Phos for Catalytic Asymmetric Alkynylation of Aromatic Aldehydes with Unexpected Reversal of Enantioselectivity (pages 1708–1718)

      Tao Song, Long-Sheng Zheng, Fei Ye, Wen-Hui Deng, Yun-Long Wei, Ke-Zhi Jiang and Li-Wen Xu

      Version of Record online: 30 APR 2014 | DOI: 10.1002/adsc.201301128

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    2. Chiral Phosphoric Acid-Catalyzed Enantioselective Three- Component Aza-Diels–Alder Reactions of Aminopyrroles and Aminopyrazoles (pages 1719–1724)

      Julien Brioche, Thibaut Courant, Lilian Alcaraz, Michael Stocks, Mark Furber, Jieping Zhu and Géraldine Masson

      Version of Record online: 9 APR 2014 | DOI: 10.1002/adsc.201400093

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    3. Regioselective Benzylation of Diols and Polyols by Catalytic Amounts of an Organotin Reagent (pages 1735–1740)

      Hengfu Xu, Yuchao Lu, Yixuan Zhou, Bo Ren, Yuxin Pei, Hai Dong and Zhichao Pei

      Version of Record online: 7 MAY 2014 | DOI: 10.1002/adsc.201301152

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    4. Tetra-n-butylammonium Bromide: A Simple but Efficient Organocatalyst for Alcohol Oxidation under Mild Conditions (pages 1741–1746)

      Xinyi Ma, Zhongfeng Li, Feijie Liu, Shengli Cao and Honghua Rao

      Version of Record online: 30 APR 2014 | DOI: 10.1002/adsc.201400100

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    5. Enantioselective Cascade Oxa-Michael–Michael Reactions of 2-Hydroxynitrostyrenes with Enones Using a Prolinol Thioether Catalyst (pages 1753–1760)

      Ai-Bao Xia, Chao Wu, Tao Wang, Yan-Peng Zhang, Xiao-Hua Du, Ai-Guo Zhong, Dan-Qian Xu and Zhen-Yuan Xu

      Version of Record online: 9 APR 2014 | DOI: 10.1002/adsc.201301114

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  6. Full Papers

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    4. Corrigendum
    5. Review
    6. Communications
    7. Full Papers
    8. Updates
    1. Electrogenerated N-Heterocyclic Carbene in Ionic Liquid: An Insight into the Mechanism of the Oxidative Esterification of Aromatic Aldehydes (pages 1773–1781)

      Gianpiero Forte, Isabella Chiarotto, Achille Inesi, Maria Antonietta Loreto and Marta Feroci

      Version of Record online: 9 APR 2014 | DOI: 10.1002/adsc.201400163

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    2. Synthesis of Quinazolinones from Alcohols via Laccase-Mediated Tandem Oxidation (pages 1789–1794)

      Marjan Heidary, Mehdi Khoobi, Sabrieh Ghasemi, Zohreh Habibi and Mohammad Ali Faramarzi

      Version of Record online: 6 MAY 2014 | DOI: 10.1002/adsc.201400103

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    3. Chiral Octahedral Complexes of Cobalt(III) as “Organic Catalysts in Disguise” for the Asymmetric Addition of a Glycine Schiff Base Ester to Activated Olefins (pages 1803–1810)

      Victor I. Maleev, Michael North, Vladimir A. Larionov, Ivan V. Fedyanin, Tatyana F. Savel'yeva, Margarita A. Moscalenko, Alexander F. Smolyakov and Yuri N. Belokon

      Version of Record online: 15 APR 2014 | DOI: 10.1002/adsc.201400091

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    4. Titanium-Catalyzed, One-Pot Synthesis of 2-Amino-3-cyano- pyridines (pages 1811–1822)

      Amila A. Dissanayake, Richard J. Staples and Aaron L. Odom

      Version of Record online: 15 APR 2014 | DOI: 10.1002/adsc.201301046

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  7. Updates

    1. Top of page
    2. Cover Pictures
    3. Contents
    4. Corrigendum
    5. Review
    6. Communications
    7. Full Papers
    8. Updates
    1. N-Alkylations of NH-Sulfoximines and NH-Sulfondiimines with Alkyl Halides Mediated by Potassium Hydroxide in Dimethyl Sulfoxide (pages 1847–1852)

      Christine M. M. Hendriks, Rebekka A. Bohmann, Marina Bohlem and Carsten Bolm

      Version of Record online: 6 MAY 2014 | DOI: 10.1002/adsc.201400193

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    2. Palladium on Carbon-Catalyzed One-Pot N-Arylindole Synthesis: Intramolecular Aromatic Amination, Aromatization, and Intermolecular Aromatic Amination (pages 1866–1872)

      Yasunari Monguchi, Takahisa Marumoto, Haruki Takamatsu, Yoshinari Sawama and Hironao Sajiki

      Version of Record online: 15 APR 2014 | DOI: 10.1002/adsc.201301168

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      Nitrile as Activating Group in the Asymmetric Bioreduction of β-Cyanoacrylic Acids Catalyzed by Ene-Reductases (pages 1878–1882)

      Christoph K. Winkler, Dorina Clay, Nikolaus G. Turrini, Horst Lechner, Wolfgang Kroutil, Simon Davies, Sebastien Debarge, Pat O'Neill, Jeremy Steflik, Mike Karmilowicz, John W. Wong and Kurt Faber

      Version of Record online: 9 APR 2014 | DOI: 10.1002/adsc.201301055

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