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High-Mobility Air-Stable n-Type Semiconductors with Processing Versatility: Dicyanoperylene-3,4:9,10-bis(dicarboximides)

Authors

  • Brooks A. Jones,

    1. Department of Chemistry, Center for Nanofabrication and Molecular Self-Assembly and the Materials Research Center, Northwestern University, 2145 Sheridan Road, Evanston IL, 60208-3113, USA, Fax: (+1) 847-491-2290
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  • Michael J. Ahrens,

    1. Department of Chemistry, Center for Nanofabrication and Molecular Self-Assembly and the Materials Research Center, Northwestern University, 2145 Sheridan Road, Evanston IL, 60208-3113, USA, Fax: (+1) 847-491-2290
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  • Myung-Han Yoon,

    1. Department of Chemistry, Center for Nanofabrication and Molecular Self-Assembly and the Materials Research Center, Northwestern University, 2145 Sheridan Road, Evanston IL, 60208-3113, USA, Fax: (+1) 847-491-2290
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  • Antonio Facchetti Dr.,

    1. Department of Chemistry, Center for Nanofabrication and Molecular Self-Assembly and the Materials Research Center, Northwestern University, 2145 Sheridan Road, Evanston IL, 60208-3113, USA, Fax: (+1) 847-491-2290
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  • Tobin J. Marks Prof.,

    1. Department of Chemistry, Center for Nanofabrication and Molecular Self-Assembly and the Materials Research Center, Northwestern University, 2145 Sheridan Road, Evanston IL, 60208-3113, USA, Fax: (+1) 847-491-2290
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  • Michael R. Wasielewski Prof.

    1. Department of Chemistry, Center for Nanofabrication and Molecular Self-Assembly and the Materials Research Center, Northwestern University, 2145 Sheridan Road, Evanston IL, 60208-3113, USA, Fax: (+1) 847-491-2290
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  • We thank DARPA (MDA972-03-1-0023) and ONR (N00014-02-1-0909, N00014-02-1-0381) for support of this research, and the Northwestern Materials Research Center (NSF-MRSEC DMR-0076097) for characterization facilities. We also thank Charlotte Stern for single-crystal X-ray diffraction data collection and Matthew Russell for aid with SEM measurements.

Abstract

original image

Viele Wege führen zu Bauelementen mit luftstabilen organischen Feldeffekttransistoren aus einer neuen Klasse äußerst elektronenarmer cyanierter Perylendiimide, die n-Ladungsträger-Beweglichkeiten bis 0.64 cm2 V−1 s−1 zeigen (siehe Bild): aus der Gasphase oder aus Lösung abgeschiedene Filme sowie BOC- und TOC-Elektrodenkonfigurationen (BOC: bottom contact, TOC: top contact).

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