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Cooperative Assembly of Three-Ring-Based Zeolite-Type Metal–Organic Frameworks and Johnson-Type Dodecahedra

Authors

  • Dr. Shou-Tian Zheng,

    1. Department of Chemistry and Biochemistry, California State University, Long Beach, 1250 Bellflower Boulevard, Long Beach, CA 90840 (USA), Fax: (+1) 562-985-8557
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  • Fan Zuo,

    1. Department of Chemistry, University of California, Riverside, CA 92521 (USA)
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  • Tao Wu,

    1. Department of Chemistry, University of California, Riverside, CA 92521 (USA)
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  • Burcin Irfanoglu,

    1. Department of Chemistry and Biochemistry, California State University, Long Beach, 1250 Bellflower Boulevard, Long Beach, CA 90840 (USA), Fax: (+1) 562-985-8557
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  • Chengtsung Chou,

    1. Department of Chemistry and Biochemistry, California State University, Long Beach, 1250 Bellflower Boulevard, Long Beach, CA 90840 (USA), Fax: (+1) 562-985-8557
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  • Ruben A. Nieto,

    1. Department of Chemistry and Biochemistry, California State University, Long Beach, 1250 Bellflower Boulevard, Long Beach, CA 90840 (USA), Fax: (+1) 562-985-8557
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  • Prof. Dr. Pingyun Feng,

    1. Department of Chemistry, University of California, Riverside, CA 92521 (USA)
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  • Prof. Dr. Xianhui Bu

    Corresponding author
    1. Department of Chemistry and Biochemistry, California State University, Long Beach, 1250 Bellflower Boulevard, Long Beach, CA 90840 (USA), Fax: (+1) 562-985-8557
    • Department of Chemistry and Biochemistry, California State University, Long Beach, 1250 Bellflower Boulevard, Long Beach, CA 90840 (USA), Fax: (+1) 562-985-8557
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  • We thank the NSF (X.B. DMR-0846958, P.F. DMR-0907175) and DOE (P.F. DE-SC0002235) for support of this work. X.B. is a Henry Dreyfus Teacher Scholar.

Abstract

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MOFs und MOPs: Die kooperative Anordnung von Indiumknoten mit vierfacher Konnektivität und zwei Liganden komplementärer Symmetrie ergibt Dreierring-basierte Metall-organische Zeolithgerüste vom NPO-Typ (NPO-Zeolith-MOFs) und Metall-organische Johnson-Polyeder (Johnson-MOPs; grau C, grün In, blau N, rot O). Die NPO-Zeolithe sind Halbleiter und photokatalytisch aktiv bei der Erzeugung von H2 aus Wasser mit UV-Licht.

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