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Selective Formation of Imines by Aerobic Photocatalytic Oxidation of Amines on TiO2

Authors

  • Dr. Xianjun Lang,

    1. Key Laboratory of Photochemistry, Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190 (China), Fax: (+86) 10-8261-6495
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  • Dr. Hongwei Ji,

    1. Key Laboratory of Photochemistry, Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190 (China), Fax: (+86) 10-8261-6495
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  • Prof. Chuncheng Chen,

    1. Key Laboratory of Photochemistry, Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190 (China), Fax: (+86) 10-8261-6495
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  • Prof. Wanhong Ma,

    1. Key Laboratory of Photochemistry, Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190 (China), Fax: (+86) 10-8261-6495
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  • Prof. Jincai Zhao

    Corresponding author
    1. Key Laboratory of Photochemistry, Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190 (China), Fax: (+86) 10-8261-6495
    • Key Laboratory of Photochemistry, Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190 (China), Fax: (+86) 10-8261-6495===

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  • Financial support from the 973 project (nos. 2010CB933503 and 2007CB613306), the NSFC (nos. 20920102034, 21077110, and 20877076,) and the CAS are gratefully acknowledged.

Abstract

original image

N→O→N: Die Titelumsetzung verläuft als zweistufiger Prozess: In einem selektiven Oxygenierungsschritt werden Aldehydintermediate gebildet, und diese werden in einem anschließenden Kondensationsschritt zu den Iminprodukten umgesetzt (siehe Schema).

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