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Highly Efficient Aerobic Oxidative Hydroxylation of Arylboronic Acids: Photoredox Catalysis Using Visible Light

Authors

  • You-Quan Zou,

    1. Key Laboratory of Pesticide & Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei 430079 (China)
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  • Dr. Jia-Rong Chen,

    1. Key Laboratory of Pesticide & Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei 430079 (China)
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  • Xiao-Peng Liu,

    1. Key Laboratory of Pesticide & Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei 430079 (China)
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  • Dr. Liang-Qiu Lu,

    1. Key Laboratory of Pesticide & Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei 430079 (China)
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  • Dr. Rebecca L. Davis,

    1. Center for Catalysis, Department of Chemistry, Aarhus University, 8000 Aarhus C (Denmark)
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  • Prof. Dr. Karl Anker Jørgensen,

    Corresponding author
    1. Center for Catalysis, Department of Chemistry, Aarhus University, 8000 Aarhus C (Denmark)
    • Center for Catalysis, Department of Chemistry, Aarhus University, 8000 Aarhus C (Denmark)
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  • Prof. Dr. Wen-Jing Xiao

    Corresponding author
    1. Key Laboratory of Pesticide & Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei 430079 (China)
    2. State Key Laboratory of Organometallic Chemistry, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, Shanghai 200032 (China)
    • Key Laboratory of Pesticide & Chemical Biology, Ministry of Education, College of Chemistry, Central China Normal University, 152 Luoyu Road, Wuhan, Hubei 430079 (China)
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  • We are grateful to the National Science Foundation of China (NO. 21072069 and 21002036) and the National Basic Research Program of China (2011CB808600) for support of this research.

Abstract

original image

Katalyse im Sichtbaren: Die Titelreaktion ermöglicht die Herstellung von funktionalisierten Phenolen und Analoga mithilfe von [Ru(bpy)3Cl2]⋅6 H2O als Photokatalysator unter sehr milden Reaktionsbedingungen. Dabei wird ein Sauerstoffatom aus molekularem Sauerstoff direkt in das Produkt eingebaut. bpy=Bipyridin.

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