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Low-Energy Selective Capture of Carbon Dioxide by a Pre-designed Elastic Single-Molecule Trap


  • Funding was provided by the U.S. Department of Energy (DOE DE-SC0001015 and DE-AR0000073). M.W. acknowledges the Postdoc Programme of the German Academic Exchange Service (DAAD) for his financial support. Special thanks go to C. Näther from the University of Kiel (Germany) for the crystallographic help on PCN-200-syn and A. Callejas-Tovar who carried out the IAST calculations. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. In this context we thank K. W. Chapman for her onsite help.


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Einzelmolekülfalle: Die einfache Aktivierung der wasserbeständigen Metall-organischen Gerüststruktur PCN-200 öffnet eine neue Route für die selektive CO2-Einlagerung durch responsive Adsorption. Der elastische CO2-Einfang wurde anhand von Adsorptionsisothermen für einzelne Komponenten und binäre Gasmischung sowie kristallographische Studien bestätigt.

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