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Rhodium or Ruthenium-Catalyzed Oxidative C[BOND]H/C[BOND]H Cross-Coupling: Direct Access to Extended π-Conjugated Systems

Authors

  • Jiaxing Dong,

    1. Key Laboratory of Green Chemistry and Technology of Ministry of Education, College of Chemistry, and State Key Laboratory of Biotherapy, West China Medical School, Sichuan University, 29 Wangjiang Road, Chengdu 610064 (PR China)
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  • Zhen Long,

    1. Key Laboratory of Green Chemistry and Technology of Ministry of Education, College of Chemistry, and State Key Laboratory of Biotherapy, West China Medical School, Sichuan University, 29 Wangjiang Road, Chengdu 610064 (PR China)
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  • Dr. Feijie Song,

    1. Key Laboratory of Green Chemistry and Technology of Ministry of Education, College of Chemistry, and State Key Laboratory of Biotherapy, West China Medical School, Sichuan University, 29 Wangjiang Road, Chengdu 610064 (PR China)
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  • Ningjie Wu,

    1. Key Laboratory of Green Chemistry and Technology of Ministry of Education, College of Chemistry, and State Key Laboratory of Biotherapy, West China Medical School, Sichuan University, 29 Wangjiang Road, Chengdu 610064 (PR China)
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  • Qiang Guo,

    1. Key Laboratory of Green Chemistry and Technology of Ministry of Education, College of Chemistry, and State Key Laboratory of Biotherapy, West China Medical School, Sichuan University, 29 Wangjiang Road, Chengdu 610064 (PR China)
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  • Prof. Dr. Jingbo Lan,

    1. Key Laboratory of Green Chemistry and Technology of Ministry of Education, College of Chemistry, and State Key Laboratory of Biotherapy, West China Medical School, Sichuan University, 29 Wangjiang Road, Chengdu 610064 (PR China)
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  • Prof. Dr. Jingsong You

    Corresponding author
    1. Key Laboratory of Green Chemistry and Technology of Ministry of Education, College of Chemistry, and State Key Laboratory of Biotherapy, West China Medical School, Sichuan University, 29 Wangjiang Road, Chengdu 610064 (PR China)
    • Key Laboratory of Green Chemistry and Technology of Ministry of Education, College of Chemistry, and State Key Laboratory of Biotherapy, West China Medical School, Sichuan University, 29 Wangjiang Road, Chengdu 610064 (PR China)
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  • This work was supported by grants from the National Basic Research Program of China (973 Program, 2011CB808600), and the National NSF of China (21025205, 20972102, 21021001, and J1103315J0104).

Abstract

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Gemischtes Doppel: Eine chemo- und regioselektive oxidative Kreuzkupplung zwischen verschiedenen (N-Heteroaryl)arenen und Heteroarenen mit doppelter C-H-Aktivierung wird beschrieben. Die Reaktion liefert unter Rhodium- oder Rutheniumkatalyse eine Reihe hoch funktionalisierter konjugierter π-Systeme.

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