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A Water Stable Metal–Organic Framework with Optimal Features for CO2 Capture

Authors

  • Prof. Qingyuan Yang,

    1. State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029 (China)
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  • Dr. Sébastien Vaesen,

    1. Thermodynamics Department, Faculté Polytechnique, Université de UMONS, Place du Parc 20, 7000 Mons (Belgium)
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  • Florence Ragon,

    1. Institut Lavoisier, UMR CNRS 8180-Université de Versailles, St Quentin en Yvelines, 45 avenue des Etats-Unis, 78035 Versailles (France)
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  • Dr. Andrew D. Wiersum,

    1. Laboratoire MADIREL, Aix-Marseille Univ. - CNRS, UMR 7246, Centre de Saint Jérôme, 13397 Marseille (France)
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  • Dong Wu,

    1. State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029 (China)
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  • Dr. Ana Lago,

    1. Institut Lavoisier, UMR CNRS 8180-Université de Versailles, St Quentin en Yvelines, 45 avenue des Etats-Unis, 78035 Versailles (France)
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  • Dr. Thomas Devic,

    1. Institut Lavoisier, UMR CNRS 8180-Université de Versailles, St Quentin en Yvelines, 45 avenue des Etats-Unis, 78035 Versailles (France)
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  • Dr. Charlotte Martineau,

    1. Institut Lavoisier, UMR CNRS 8180-Université de Versailles, St Quentin en Yvelines, 45 avenue des Etats-Unis, 78035 Versailles (France)
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  • Dr. Francis Taulelle,

    1. Institut Lavoisier, UMR CNRS 8180-Université de Versailles, St Quentin en Yvelines, 45 avenue des Etats-Unis, 78035 Versailles (France)
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  • Dr. Philip L. Llewellyn,

    1. Laboratoire MADIREL, Aix-Marseille Univ. - CNRS, UMR 7246, Centre de Saint Jérôme, 13397 Marseille (France)
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  • Dr. Hervé Jobic,

    1. Institut de Recherches sur la Catalyse et l'Environnement de Lyon, Université de Lyon, CNRS, 2. Av. A. Einstein, 69626 Villeurbanne (France)
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  • Prof. Chongli Zhong,

    1. State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, Beijing, 100029 (China)
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  • Dr. Christian Serre,

    Corresponding author
    1. Institut Lavoisier, UMR CNRS 8180-Université de Versailles, St Quentin en Yvelines, 45 avenue des Etats-Unis, 78035 Versailles (France)
    • Christian Serre, Institut Lavoisier, UMR CNRS 8180-Université de Versailles, St Quentin en Yvelines, 45 avenue des Etats-Unis, 78035 Versailles (France)

      Guy De Weireld, Thermodynamics Department, Faculté Polytechnique, Université de UMONS, Place du Parc 20, 7000 Mons (Belgium)

      Guillaume Maurin, Institut Charles Gerhardt Montpellier, UMR CNRS 5253, UM2, ENSCM, Place E. Bataillon, 34095 Montpellier cedex 05 (France)

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  • Prof. Guy De Weireld,

    Corresponding author
    1. Thermodynamics Department, Faculté Polytechnique, Université de UMONS, Place du Parc 20, 7000 Mons (Belgium)
    • Christian Serre, Institut Lavoisier, UMR CNRS 8180-Université de Versailles, St Quentin en Yvelines, 45 avenue des Etats-Unis, 78035 Versailles (France)

      Guy De Weireld, Thermodynamics Department, Faculté Polytechnique, Université de UMONS, Place du Parc 20, 7000 Mons (Belgium)

      Guillaume Maurin, Institut Charles Gerhardt Montpellier, UMR CNRS 5253, UM2, ENSCM, Place E. Bataillon, 34095 Montpellier cedex 05 (France)

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  • Prof. Guillaume Maurin

    Corresponding author
    1. Institut Charles Gerhardt Montpellier, UMR CNRS 5253, UM2, ENSCM, Place E. Bataillon, 34095 Montpellier cedex 05 (France)
    • Christian Serre, Institut Lavoisier, UMR CNRS 8180-Université de Versailles, St Quentin en Yvelines, 45 avenue des Etats-Unis, 78035 Versailles (France)

      Guy De Weireld, Thermodynamics Department, Faculté Polytechnique, Université de UMONS, Place du Parc 20, 7000 Mons (Belgium)

      Guillaume Maurin, Institut Charles Gerhardt Montpellier, UMR CNRS 5253, UM2, ENSCM, Place E. Bataillon, 34095 Montpellier cedex 05 (France)

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  • This research was funded by the European Community’s Seventh Framework Programme (FP7/2007-2013) under grant agreement No. 228862, the Natural Science Foundation of China (21136001, 21276009), and the Beijing Nova Program (No. 2008B15). We thank Dr. M. M. Koza for his help during the measurements on the IN6 spectrometer at the Institut Laue Langevin, Grenoble, France.

Abstract

original image

One flue over the cuckoo's nest: A novel porous Zr-based MOF combining a high chemical stability, easy “green” synthesis and scalability is prepared. This material incorporating carboxylic functions on its organic linkers has thermodynamically and kinetically very promising properties for CO2 capture from post-combustion flue gas under real working conditions.

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