An In Situ Carbonaceous Mesoporous Template for the Synthesis of Hierarchical ZSM-5 Zeolites by One-Pot Steam-Assisted Crystallization

Authors

  • Dr. Yudian Song,

    1. State Key Laboratory of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences, No.1295 Ding-xi Road, Shanghai, 200050 (P.R. China), Fax: (+86) 21-5241-3122
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  • Dr. Zile Hua,

    1. State Key Laboratory of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences, No.1295 Ding-xi Road, Shanghai, 200050 (P.R. China), Fax: (+86) 21-5241-3122
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  • Dr. Yan Zhu,

    1. State Key Laboratory of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences, No.1295 Ding-xi Road, Shanghai, 200050 (P.R. China), Fax: (+86) 21-5241-3122
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  • Dr. Xiaoxia Zhou,

    1. State Key Laboratory of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences, No.1295 Ding-xi Road, Shanghai, 200050 (P.R. China), Fax: (+86) 21-5241-3122
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  • Wei Wu,

    1. State Key Laboratory of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences, No.1295 Ding-xi Road, Shanghai, 200050 (P.R. China), Fax: (+86) 21-5241-3122
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  • Linlin Zhang,

    1. State Key Laboratory of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences, No.1295 Ding-xi Road, Shanghai, 200050 (P.R. China), Fax: (+86) 21-5241-3122
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  • Prof. Jianlin Shi

    Corresponding author
    1. State Key Laboratory of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences, No.1295 Ding-xi Road, Shanghai, 200050 (P.R. China), Fax: (+86) 21-5241-3122
    • State Key Laboratory of High Performance Ceramics and Superfine Microstructures, Shanghai Institute of Ceramics, Chinese Academy of Sciences, No.1295 Ding-xi Road, Shanghai, 200050 (P.R. China), Fax: (+86) 21-5241-3122

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Abstract

original image

Blackened catalyst: Zeolites with large external surface area and mesopore volume were synthesized by a one-pot templating strategy, in which the crystallization proceeded concurrently with in situ carbonization templating to produce a mesoporous structure. The hierarchical materials exhibited superior catalytic performance over conventional zeolites in Friedel–Crafts acylation of anisole.

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