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Keywords:

  • lanthanoids;
  • ligand field theory;
  • magnetic properties;
  • phthalocyanines;
  • single-molecule magnets
Thumbnail image of graphical abstract

A single magnet in a triple decker! TbIII–phthalocyaninate triple-decker 1, which has a center of symmetry, showed two magnetic relaxation processes in the low-temperature region in the presence of a direct current (dc) magnetic field. These results suggest that the single-molecule magnet/magnetic properties of 1 undergo a significant transition in a dc magnetic field.