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Keywords:

  • chelates;
  • density functional calculations;
  • electronic structure;
  • N ligands;
  • radical ions;
  • ruthenium
Thumbnail image of graphical abstract

Redox-active ligands: Structural, spectroscopic, and theoretical studies of ruthenium(II) complexes bearing 2-(2-nitrosoaryl)pyridine ligands and their reduced analogues reveals the redox noninnocence of 2-(2-nitrosoaryl)pyridine (see scheme).