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The cover picture shows the binary chalcogenidotetrelate building blocks [TE4]4– and [(RT)4E6] that were used to generate the rich variety of compounds depicted around them. In their perspective article Dehnen et al. describe a stepwise coordination chemistry approach, allowing the sequential formation of multinary chalcogenidometallates and intricate organofunctionalized clusters, starting from these simple precursors The article outlines structure types, factors influencing the formation of specific structures and the properties of the resulting materials, and can be found on pages 2425 ff.