A multiple year-round study of atmospheric dimethyl sulfide (DMS) (from December 1998 to April 2003) as well as sulfur-derived aerosols (methanesulfonic acid (MSA) and non-sea-salt sulfate) (from March 1991 to February 2003) was conducted at Dumont d'Urville, coastal Antarctica. The three sulfur-derived species exhibit a seasonal cycle characterized by maxima in midsummer (January). Whereas the interannual variability of winter levels remains low, a strong interannual variability is shown in summer, particularly for DMS and MSA, and to a lesser extent for non-sea-salt sulfate. Over the 1998–2003 time period, January 2002 stands out with high values for all sulfur species. These interannual variabilities of atmospheric summer levels are examined in the light of seawater chlorophyll a content derived from Sea-viewing Wide Field-of-view Sensor (SeaWiFS) data (themselves compared to field measurements made south of 60°S), oceanic DMS levels estimated from chlorophyll a SeaWiFS data, and various sea-ice indices.