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Auxiliary material for this article contains additional details of the atmospheric transport and chemistry used in this work and an analysis of the optimized model output.

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FilenameFormatSizeDescription
grl25320-sup-0001-readme.txtplain text document3Kreadme.txt
grl25320-sup-0002-txts01.txtplain text document4KText S1. Interannually varying temperature and transport in the box model.
grl25320-sup-0003-txts02.txtplain text document1KText S2. Comparison of optimized box model methane mole fractions and AGAGE/CSIRO measurements.
grl25320-sup-0004-txts03.txtplain text document0KText S3. Comparison of optimized box model methyl chloroform mole fractions and AGAGE/CSIRO measurements.
grl25320-sup-0005-txts04.txtplain text document2KText S4. Optimized error covariance matrix analysis.
grl25320-sup-0006-fs01.epsPS document94KFigure S1. Difference between AGAGE/CSIRO measurements and modeled semi-hemispheric and hemispheric mole fractions with optimized emissions.
grl25320-sup-0007-fs02.epsPS document59KFigure S2. Residual CH3CCl3 mole fraction for optimized OH fields.
grl25320-sup-0008-fs03.epsPS document29KFigure S3. Mean covariance between each monthly emission rate and previous/subsequent months for each box and average covariance between pairs of boxes for each calendar month.
grl25320-sup-0009-t01.txtplain text document1KTab-delimited Table 1.

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