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Figure S1. A. Titration of 25 μM ArgenCast-1 with AgClO4 in CH3CN. B. Difference curve C. Binding isotherm. Error bars represent the variance in the measurements over three trials.

Figure S2. A. Titration of 25 μM ArgenCast-1 with Hg2ClO4 in CH3CN. B. Difference curve C. Binding isotherm. Error bars represent the variance in the measurements over three trials.

Figure S3. A.Titration of 25 μM ArgenCast-1 with AgClO4 in MeOH. B. Difference curve C. Binding isotherm. Error bars represent the variance in the measurements over three trials.

Figure S4. A. Titration of 25 μM ArgenCast-1 with (CH3CN)4CuPF6 in MeOH. B. Difference curve. C. Binding isotherm. Error bars represent the variance in the measurements over three trials.

Figure S5. A. Titration of 25 μM ArgenCast-1 with AgClO4 in buffer. B. Difference curve. C. Binding isotherm. Error bars represent the variance in the measurements over three trials.

Figure S6. A. Titration of 25 μM ArgenUnc-1 with AgClO4 in CH3CN. B. Difference curve. C. Binding isotherm. Error bars represent the variance in the measurements over three trials.

Figure S7. A. Titration of 25 μM ArgenUnc-1 with Hg2ClO4 in CH3CN. B. Difference curve. C. Binding isotherm. Error bars represent the variance in the measurements over three trials.

Figure S8. A. Titration of 25 μM ArgenUnc-1 with AgClO4 in MeOH. B. Difference curve. C. Binding isotherm. Error bars represent the variance in the measurements over three trials.

Figure S9. A. Titration of 25 μM ArgenUnc-1 with (CH3CN)4CuPF6 in MeOH. B. Difference curve. C. Binding isotherm. Error bars represent the variance in the measurements over three trials.

Figure S10. A. Titration of 25 μM ArgenUnc-1 with AgClO4 in buffer. B. Difference curve. C. Binding isotherm. Error bars represent the variance in the measurements over three trials.

Figure S11. Photolysis of 25 μM ArgenCast-1 in MeCN using a 8 W lamps photo reactor source at 350 nm.

Figure S12. Photolysis of 25 μM ArgenCast-1 in MeOH using a 8 W lamps photo reactor source at 350 nm.

Figure S13. Photolysis of 25 μM ArgenCast-1 in buffer using a 8 W lamps photo reactor source at 350 nm.

Figure S14. Photolysis of 25 μM ArgenCast-2 in MeCN using a 8 W lamps photo reactor source at 350 nm.

Figure S15. Photolysis of 25 μM ArgenCast-2 in MeOH using a 8 W lamps photoreactor source at 350 nm.

Figure S16. Photolysis of 25 μM ArgenCast-2 in buffer using a 8 W lamps photoreactor source at 350 nm.

Figure S17. Photolysis of 25 μM ArgenCast-3 in MeCN using a 8 W lamps photoreactor source at 350 nm.

Figure S18. Photolysis of 25 μM ArgenCast-3 in MeOH using a 8 W lamps photoreactor source at 350 nm.

Figure S19. Photolysis of 25 μM ArgenCast-3 in buffer using a 8 W lamps photoreactor source at 350 nm.

Figure S20. Photolysis of 25 μM ArgenCast-1 in the presence of 25 μM AgClO4 (1 Eq) in MeCN using a 8 W lamps photoreactor source at 350 nm.

Figure S21. Photolysis of 25 μM ArgenCast-1 in the presence of 25 μM AgClO4 (1 Eq) in MeOH using a 8 W lamps photoreactor source at 350 nm.

Figure S22. Photolysis of 25 μM ArgenCast-1 in the presence of 25 μM AgClO4 (1 Eq) in buffer using a 8 W lamps photoreactor source at 350 nm.

Figure S23. Photolysis of 25 μM ArgenCast-1 in the presence of 25 μM (CH3CN)4CuPF6 (1 Eq) in MeOH using a 8 W lamps photoreactor source at 350 nm.

Figure S24. Photolysis of 25 μM ArgenCast-2 in the presence of 25 μM AgClO4 (1 Eq) in MeCN using a 8 W lamps photoreactor source at 350 nm.

Figure S25. Photolysis of 25 μM ArgenCast-2 in the presence of 25 μM AgClO4 (1 Eq) in MeOH using a 8 W lamps photoreactor source at 350 nm.

Figure S26. Photolysis of 25 μM ArgenCast-2 in the presence of 25 μM AgClO4 (1 Eq) in buffer using a 8 W lamps photoreactor source at 350 nm.

Figure S27. Photolysis of 25 μM ArgenCast-2 in the presence of 25 μM (CH3CN)4CuPF6 (1 Eq) in MeOH using a 8 W lamps photoreactor source at 350 nm.

Figure S28. Photolysis of 25 μM ArgenCast-3 in the presence of 25 μM AgClO4 (1 Eq) in MeCN using a 8 W lamps photoreactor source at 350 nm.

Figure S29. Photolysis of 25 μM ArgenCast-3 in the presence of 25 μM AgClO4 (1 Eq) in MeOH using a 8 W lamps photoreactor source at 350 nm.

Figure S30. Photolysis of 25 μM ArgenCast-3 in the presence of 25 μM (CH3CN)4CuPF6 (1 Eq) in MeOH using a 8 W lamps photoreactor source at 350 nm.

Figure S31. 1H and 13C NMR for ArgenCast-1.

Figure S32. 1H and 13C NMR for ArgenUNC-1.

Figure S33. 1H and 13C NMR for ArgenCast-2.

Figure S34. 1H and 13C NMR for ArgenCast-3.

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