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Jordan L. Arthur, Saul H. Lapidus, Curtis E. Moore, Arnold L. Rheingold, Peter W. Stephens and Joel S. Miller N,7,7-Tricyanoquinomethanimine (TCQMI) Based Organic Magnetic Materials Advanced Functional Materials 22

Version of Record online: 14 MAR 2012 | DOI: 10.1002/adfm.201101937

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A new family of organic magnets with N,7, 7-tricyanoquinomethanimine (TCQMI) is reported. [FeIII(C5Me5)2]•+[TCQMI]•− forms parallel chains of alternating radical cations/anions and orders at 3.4 K as a weak ferromagnet. Amorphous M[TCQMI]2z CH2Cl2 (M = V, Fe) have μ4-[TCQMI]•−, and the Fe compound is a weak ferromagnet at ≈4 K, whereas the V compound does not magnetically order.

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