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Thomas Tischer, Anja S. Goldmann, Katharina Linkert, Vanessa Trouillet, Hans G. Börner and Christopher Barner-Kowollik Modular Ligation of Thioamide Functional Peptides onto Solid Cellulose Substrates Advanced Functional Materials 22

Version of Record online: 4 JUN 2012 | DOI: 10.1002/adfm.201200266

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Peptide-cellulose hybrid materials are generated via mild hetero Diels-Alder (HDA) cycloaddition to graft thioamide functional oligopeptides onto solid cellulose substrates bearing highly reactive cyclopentadienyl moieties. Oligopeptides (including antimicrobial tritrpticin) are functionalized employing strongly electron deficient thiocarbonyl thio compounds resulting in biomacromolecules bearing a thioamide endgroup. In-depth investigations in solution and on the solid peptide functional substrate were performed confirming a highly efficient grafting process.

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