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Young-Si Jun, Eun Zoo Lee, Xinchen Wang, Won Hi Hong, Galen D. Stucky and Arne Thomas From Melamine-Cyanuric Acid Supramolecular Aggregates to Carbon Nitride Hollow Spheres Advanced Functional Materials 23

Article first published online: 26 FEB 2013 | DOI: 10.1002/adfm.201203732

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Simple molecular engineering of triazine precursors enables simultaneous optimization of the texture and photoelectric properties of graphitic carbon nitride (g-CN). Thermolysis of flower-like supramolecular aggregates of melamine and cyanuric acid yields the formation of mesoporous g-CN hollow spheres with the typical nanosheet-type structure preserved in the microspheres. Such structures are highly active in the photocatalytic degradation of organic pollutants.

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