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David B. Mitzi Solution Processing of Chalcogenide Semiconductors via Dimensional Reduction Advanced Materials 21

Version of Record online: 21 APR 2009 | DOI: 10.1002/adma.200802027

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One approach to improving the solubility of inorganic semiconductors for film deposition involves breaking up the extended framework into discrete anionic moieties, separated by small and volatile cationic species (so-called “dimensional reduction” of the inorganic framework), resulting in a soluble precursor. Using this approach and a reactive hydrazine solvent, high quality metal chalcogenide films are deposited for applications including thin-film transistors and solar cells.

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