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Suhao Wang, Michael Kappl, Ingo Liebewirth, Maren Müller, Katrin Kirchhoff, Wojciech Pisula and Klaus Müllen Organic Field-Effect Transistors based on Highly Ordered Single Polymer Fibers Advanced Materials 24

Article first published online: 15 DEC 2011 | DOI: 10.1002/adma.201103057

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Ultrahigh-mobility organic field-effect transistors (OFETs) based on a CDT-BTZ donor-acceptor copolymer are realized by reaching high molecular order and pronounced alignment in single fibers within a short OFET channel via solution processing. The macromolecules directionally self-assemble in a quasi crystal-like order in the fibers providing in this way an unhindered charge carrier pathway with mobilities as high as 5.5 cm2 V−1 s−1.

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