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Felix Schlosser, Michael Moos, Christoph Lambert and Frank Würthner Redox-switchable Intramolecular π−π-Stacking of Perylene Bisimide Dyes in a Cyclophane Advanced Materials 25

Article first published online: 16 JUL 2012 | DOI: 10.1002/adma.201201266

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Molecular actuation by stepwise electrochemical reduction is demonstrated for a cyclophane that exhibits a pronounced conformational transition from a closed cavity with cofacially stacked PBIs in the neutral state to an expanded open cavity in the three- and fourfold reduced state.

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