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Shinto Varghese, Seong-Jun Yoon, Eva M. Calzado, Santiago Casado, Pedro G. Boj, María A. Díaz-García, Roland Resel, Roland Fischer, Begoña Milián-Medina, Reinhold Wannemacher, Soo Young Park and Johannes Gierschner Stimulated Resonance Raman Scattering and Laser Oscillation in Highly Emissive Distyrylbenzene-Based Molecular Crystals Advanced Materials 24

Version of Record online: 12 OCT 2012 | DOI: 10.1002/adma.201202525

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Three-in-one: A novel distyrylbenzene-based material forms J-type aggregates in single crystals with highly polarized and bright red emission, giving rise to optical gain narrowing, for which different mechanisms (amplified spontaneous emission, laser emission and stimulated resonance Raman scattering) are observed. These are correlated with the favorable intrinsic and macroscopic properties of the crystal, in particular to the orientation of the molecules to the crystal surface.

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