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Myung-Hyun Ryou, Jangbae Kim, Inhwa Lee, Sunjin Kim, You Kyeong Jeong, Seonki Hong, Ji Hyun Ryu, Taek-Soo Kim, Jung-Ki Park, Haeshin Lee and Jang Wook Choi Mussel-Inspired Adhesive Binders for High-Performance Silicon Nanoparticle Anodes in Lithium-Ion Batteries Advanced Materials 25

Article first published online: 27 DEC 2012 | DOI: 10.1002/adma.201203981

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Conjugation of mussel-inspired catechol groups to various polymer backbones results in materials suitable as silicon anode binders. The unique wetness-resistant adhesion provided by the catechol groups allows the silicon nanoparticle electrodes to maintain their structure throughout the repeated volume expansion and shrinkage during lithiation cycling, thus facilitating substantially improved specific capacities and cycle lives of lithium-ion batteries.

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