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Shubin Yang, Yongji Gong, Jinshui Zhang, Liang Zhan, Lulu Ma, Zheyu Fang, Robert Vajtai, Xinchen Wang and Pulickel M. Ajayan Exfoliated Graphitic Carbon Nitride Nanosheets as Efficient Catalysts for Hydrogen Evolution Under Visible Light Advanced Materials 25

Version of Record online: 1 MAR 2013 | DOI: 10.1002/adma.201204453

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Graphitic carbon nitride nanosheets are extracted, produced via simple liquid-phase exfoliation of a layered bulk material, g-C3N4. The resulting nanosheets, having ≈2 nm thickness and N/C atomic ratio of 1.31, show an optical bandgap of 2.65 eV. The carbon nitride nanosheets are demonstrated to exhibit excellent photocatalytic activity for hydrogen evolution under visible light.

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