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Takahiro Kakuta, Yoshinori Takashima, Masaki Nakahata, Miyuki Otsubo, Hiroyasu Yamaguchi and Akira Harada Preorganized Hydrogel: Self-Healing Properties of Supramolecular Hydrogels Formed by Polymerization of Host–Guest-Monomers that Contain Cyclodextrins and Hydrophobic Guest Groups Advanced Materials 25

Version of Record online: 19 FEB 2013 | DOI: 10.1002/adma.201205321

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Supramolecular hydrogels formed by a host-guest interaction show self-healing properties. The cube-shaped hydrogels with β-cyclodextrin and adamantane guest molecules mend after being broken. The hydrogels sufficiently heal to form a single gel, and the initial strength is restored. Although contact between a freshly cut and uncut surface does not mend the gels, two freshly cut surfaces selectively mend.

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