Xiang Zhu, Chengcheng Tian, Songhai Chai, Kimberly Nelson, Kee Sung Han, Edward W. Hagaman, Gabriel M. Veith, Shannon M. Mahurin, Honglai Liu and Sheng Dai New Tricks for Old Molecules: Development and Application of Porous N-doped, Carbonaceous Membranes for CO2 Separation Advanced Materials 25
A new strategy is successfully applied to “old” acetyl compounds. A free-standing, porous, N-doped carbonaceous membrane is facilely prepared from the thermal treatment of a pyrrole-ring-containing polymeric membrane based on the superacid-catalyzed copolymerization of acetyl monomers. An exceptional ideal CO2/N2 permselectivity of 43.2 is achieved with a good CO2 permeability of 1149.3 Barrer, exceeding the recent upper bound for CO2/N2.
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