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Shen Yu, Rongchun Zhang, Qiang Wu, Tiehong Chen and Pingchuan Sun Bio-Inspired High-Performance and Recyclable Cross-Linked Polymers Advanced Materials 25

Version of Record online: 17 JUL 2013 | DOI: 10.1002/adma.201301513

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Bio-inspired molecular design and synthesis of high-performance and recyclable cross-linked polymers is reported. Reversible cross-links between hard segments are incorporated into linear segmented polyurethane via Diels-Alder reaction between maleimide pendant group and furan cross-linker. The materials form hierarchical structure and exhibit excellent properties with high stiffness, strength and toughness, and can be easily thermally reshaped and re-mended.

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