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Shumei Chen, Winghan Wong, Yuebun Pun, Kokwai Cheah and Guixin Li Surface Plasmon-Enhanced Third Harmonic Generation from Gold–Polymer Hybrid Plasmonic Crystal Advanced Optical Materials 1

Article first published online: 26 MAY 2013 | DOI: 10.1002/adom.201300144

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A nonlinear optical plasmonic crystal is designed by integrating an organic active medium with a large optical nonlinearity into a conventional plasmonic nanostructure. The surface plasmon-enhanced third harmonic generation (THG) from the metal–organic hybrid plasmonic crystal is experimentally demonstrated. The metal–organic hybrid configuration provides new concepts to develop novel nonlinear optical devices with subwavelength electromagnetic-wave confinement.

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