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Coleman X. Kronawitter, Zhixun Ma, Dongfang Liu, Samuel S. Mao and Bonnie R. Antoun Engineering Impurity Distributions in Photoelectrodes for Solar Water Oxidation Advanced Energy Materials 2

Article first published online: 16 NOV 2011 | DOI: 10.1002/aenm.201100425

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A strategy is introduced to decouple the optical absorption and electronic transport processes required for operation of oxide photoelectrodes in photoelectrochemical cells. Results indicate optical absorption at visible wavelengths and the related water photo-oxidation efficiencies can be enhanced by spatially segregating the functional impurity concentrations that facilitate their associated physical processes.

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