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Wesley A. Henderson, Daniel M. Seo, Qian Zhou, Paul D. Boyle, Joon-Ho Shin, Hugh C. De Long, Paul C. Trulove and Stefano Passerini An Alternative Ionic Conductivity Mechanism for Plastic Crystalline Salt–Lithium Salt Electrolyte Mixtures Advanced Energy Materials 2

Article first published online: 7 MAY 2012 | DOI: 10.1002/aenm.201200130

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The phase behavior and conductivity of mixtures of the plastic crystalline salt Et4NTFSI with LiTFSI are extensively characterized. The formation of a low-melting mixed-salt crystalline phase (and the corresponding eutectic system) in this mixture and related mixtures suggests that an alternative conductivity mechanism not based on solid-state diffusion is operable in such mixtures.

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