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Sangkyu Lee, Jaehwan Ha, Huanyu Cheng, Jung Woo Lee, Tae Sik Jang, Yeon-Gil Jung, Yonggang Huang, John A. Rogers and Ungyu Paik Surface-Coverage-Dependent Cycle Stability of Core-Shell Nanostructured Electrodes for Use in Lithium Ion Batteries Advanced Energy Materials 4

Article first published online: 31 JUL 2013 | DOI: 10.1002/aenm.201300472

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The relationship between surface coverage of the shell layer in core-shell nanostructured electrodes and the resulting electrochemical performance of the electrodes is described. Systematic studies and theoretical modeling reveal that partially covered core-shell nanostructured electrodes are beneficial to release the stress induced by lithiation and delithiation, leading to the excellent cycle performance without any capacity fading up to 50 cycles.

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