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Simone Fabiano, Scott Himmelberger, Martin Drees, Zhihua Chen, Rashid M. Altamimi, Alberto Salleo, Maria Antonietta Loi and Antonio Facchetti Charge Transport Orthogonality in All-Polymer Blend Transistors, Diodes, and Solar Cells Advanced Energy Materials 4

Version of Record online: 11 NOV 2013 | DOI: 10.1002/aenm.201301409

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Polymer aggregation and phase separation of polymer–polymer blends are effectively tuned from self-stratified to laterally phase-separated by adjusting the relative solubility of the two polymers in the mixture. This is found to dramatically alter the charge transport characteristics from a preferential in-plane to an out-of-plane direction, revealing the critical dependence of the resulting device performance on the film morphology and structure of the active layer.

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