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Allan K. Poulsen, Annette Rompel and Christine J. McKenzie Water Oxidation Catalyzed by a Dinuclear Mn Complex: A Functional Model for the Oxygen-Evolving Center of Photosystem II Angewandte Chemie International Edition 44

Version of Record online: 5 OCT 2005 | DOI: 10.1002/anie.200502114

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A highly specific and catalytic oxidation of water occurs when using a dinuclear Mn complex of a mononegative carboxylate-containing pentadentate ligand (see scheme). Isotope-labeling experiments coupled with membrane inlet mass spectrometry show that one oxygen atom in the evolved O2 molecule is derived from water and the other from the oxidant.

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