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Sven Rau, Bernhard Schäfer, Dieter Gleich, Ernst Anders, Manfred Rudolph, Manfred Friedrich, Helmar Görls, William Henry and Johannes G. Vos A Supramolecular Photocatalyst for the Production of Hydrogen and the Selective Hydrogenation of Tolane Angewandte Chemie International Edition 45

Version of Record online: 17 AUG 2006 | DOI: 10.1002/anie.200600543

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Light-driven metallo-organic catalysis: Intramolecular photoelectron transfer in the heterodinuclear complex 1 facilitates the photocatalytic production of hydrogen and the selective hydrogenation of tolane to give cis-stilbene. All three well-coordinated parts of the supramolecular system are essential: the (tbbpy)2Ru fragment as a photoactive unit, the redox-active bridging ligand as an electron relay and storage site, and the palladium as a catalytically active center.

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