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Philip L. Llewellyn, Sandrine Bourrelly, Christian Serre, Yaroslav Filinchuk and Gérard Férey How Hydration Drastically Improves Adsorption Selectivity for CO2 over CH4 in the Flexible Chromium Terephthalate MIL-53 Angewandte Chemie International Edition 45

Article first published online: 20 OCT 2006 | DOI: 10.1002/anie.200602278

Thumbnail image of graphical abstract

Taking a deep breath: The hydrated form of the microporous metal organic framework MIL-53(Cr) performs better than the dehydrated form for the selectivity binding of carbon dioxide over methane (see graph). The polarity of the adsorbed gas is thought to play a role in inducing framework flexibility and the breathing of the pores.

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