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Wei Zhuang, Tomoyuki Hayashi and Shaul Mukamel Coherent Multidimensional Vibrational Spectroscopy of Biomolecules: Concepts, Simulations, and Challenges Angewandte Chemie International Edition 48

Version of Record online: 4 MAY 2009 | DOI: 10.1002/anie.200802644

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Good vibrations: The vibrational response of complex molecules to sequences of infrared pulses provides novel femtosecond snapshots of their structure and dynamics. This technique, which is the optical analogue of multidimensional NMR spectroscopy, gives correlation plots of motions during controlled time intervals between pulses that are applied to study protein folding, chirality, hydrogen-bonding, phospholipid membranes, and chemical exchange.

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