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Bryon Simmons, Abbas M. Walji and David W. C. MacMillan Cycle-Specific Organocascade Catalysis: Application to Olefin Hydroamination, Hydro-oxidation, and Amino-oxidation, and to Natural Product Synthesis Angewandte Chemie International Edition 48

Version of Record online: 11 MAY 2009 | DOI: 10.1002/anie.200900220

Thumbnail image of graphical abstract

United in effort: The combined application of iminium (Im) and enamine (En) catalysts can effect a range of valuable asymmetric transformations including 1,2-hydroamination, -hydro-oxidation, and -amino-oxidation of olefins (see picture). An enantioselective organocascade catalysis was also applied in the synthesis of a complex natural product.

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