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Masayuki Kobayashi, Takeshi Suda, Prof. Dr. Keiichi Noguchi and Prof. Dr. Ken Tanaka Enantioselective Construction of Bridged Multicyclic Skeletons: Intermolecular [2+2+2] Cycloaddition/Intramolecular Diels–Alder Reaction Cascade Angewandte Chemie International Edition 50

Article first published online: 11 JAN 2011 | DOI: 10.1002/anie.201004150

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Bridging a gap: A cationic rhodium(I)/ligand complex catalyzes the title reaction of alkynes and amide-linked 1,5-dienes, leading to bridged multicyclic compounds, with high chemo-, regio-, and enantioselectivity (see scheme; Bn=benzyl).

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