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Dr. Tae-Hyun Bae, Jong Suk Lee, Dr. Wulin Qiu, Prof. Dr. William J. Koros, Prof. Dr. Christopher W. Jones and Prof. Dr. Sankar Nair A High-Performance Gas-Separation Membrane Containing Submicrometer-Sized Metal–Organic Framework Crystals Angewandte Chemie International Edition 49

Version of Record online: 16 NOV 2010 | DOI: 10.1002/anie.201006141

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Well matched: Submicrometer-sized metal–organic framework (MOF) crystals (ZIF-90) were synthesized by a nonsolvent-induced crystallization technique and incorporated in mixed-matrix gas-separation membranes. ZIF-90/6FDA-DAM membranes (empty pink circle; beyond the upper bound for polymer membranes) show unprecedented high performance for CO2/CH4 separation by a MOF-based membrane. The key is the combination of the highly selective MOF and a highly permeable polymer.

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