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Dr. Sarah L. Poe and Prof. Dr. James P. Morken A Boron-Based Synthesis of the Natural Product (+)-trans-Dihydrolycoricidine Angewandte Chemie International Edition 50

Version of Record online: 31 MAR 2011 | DOI: 10.1002/anie.201007135

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Diastereoselective diboration results in the highly selective 1,4-dihydroxylation of chiral cyclohexadienes (see scheme). Together with the catalytic enantioselective conjugate allylboration, the diene diboration facilitates the asymmetric synthesis of the cytotoxic agent (+)-trans-dihydrolycoricidine (1). pin=pinacol.

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