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Dr. Jun Pan, Mingjuan Su and Prof. Dr. Stephen L. Buchwald Palladium(0)-Catalyzed Intermolecular Amination of Unactivated C sp 3[BOND]H Bonds Angewandte Chemie International Edition 50

Version of Record online: 2 AUG 2011 | DOI: 10.1002/anie.201102880

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Filling out the space: The title reaction of unactivated Cmath image[BOND]H bonds using aryl amines as the nitrogen source is disclosed (see scheme; dba=dibenzylideneacetone, Tf=trifluoromethanesulfonyl). Either the C[BOND]N cross-coupling product or the C[BOND]H amination product could be accessed selectively by adjusting the steric environment of the substrate.

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