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Jane Panteleev, Lei Zhang and Prof. Dr. Mark Lautens Domino Rhodium-Catalyzed Alkyne Arylation/Palladium-Catalyzed N Arylation: A Mechanistic Investigation Angewandte Chemie International Edition 50

Article first published online: 24 AUG 2011 | DOI: 10.1002/anie.201103692

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It takes two to tango: A domino multicatalytic synthesis of dihydroquinolines is realized, wherein the products of a rhodium-catalyzed arylation of alkynes are cyclized by a palladium-promoted C[BOND]N cross-coupling (see scheme). The combination of catalysts with potentially exchangeable ligands is remarkable as each metal–ligand combination affords specific reactivity and selectivity.

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