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Dr. Dirk Hollmann, Felix Gärtner, Prof. Dr. Ralf Ludwig, Enrico Barsch, Dr. Henrik Junge, Dr. Matthias Blug, Dr. Sascha Hoch, Prof. Dr. Matthias Beller and Prof. Dr. Angelika Brückner Insights into the Mechanism of Photocatalytic Water Reduction by DFT-Supported In Situ EPR/Raman Spectroscopy Angewandte Chemie International Edition 50

Version of Record online: 10 AUG 2011 | DOI: 10.1002/anie.201103710

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Light on the water: The coupling of Raman and EPR spectroscopy was crucial in the study of the activation, operation, and deactivation steps in the light-driven splitting of water catalyzed by iridium and iron. The results may provide the foundation for improved water-reduction catalysts. IrPS=iridium photosensitizer, TEA=triethylamine.

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