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Quan Cai, Chao Zheng, Jun-Wei Zhang and Prof. Dr. Shu-Li You Enantioselective Michael/Mannich Polycyclization Cascade of Indolyl Enones Catalyzed by Quinine-Derived Primary Amines Angewandte Chemie International Edition 50

Article first published online: 26 JUL 2011 | DOI: 10.1002/anie.201103937

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Three′s a crowd: The title reaction provides a tetracylic core bearing three chiral centers (see scheme; Ts=4-toluenesulfonyl) with excellent enantioselectivity and good diastereoselectivity. The reaction was used to efficiently construct the (+)-kreysiginine skeleton.

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